4.8 Thermal effects: thermo-optic shifts, thermal lenses, ring bistability
L1 Phenomenon
Heat changes lithium niobate's extraordinary index 5 to 11 times more than its ordinary index, depending on wavelength and source (table below; thermo-optic coefficient). A ring resonator heated by its own light shifts to longer wavelength, so a laser sweeping upward drags the resonance with it and the transmission dip turns into a triangle (thermal triangle). A strong beam in a bulk crystal heats its own path and builds a lens.
- dne/dT at λ, T
- 3.75e−05 /K
- Moretti 632 nm e / o
- outside 300-515 K
- λ
- 1.550 µm
Thesis example (10 W, w 150 µm, 0.005 cm−1, 20 mm, 100 °C, 5 W/(m K)): 61 mm from its own formula with Moretti dne/dT at 632 nm; the thesis states about 100 mm. Which dn/dT it used is not stated.
A crystal that becomes a lens
absorbed power heats the beam path; dn/dT > 0 focuses- Focal length
- 7.4e+01 mm
- f / L (formula assumes f >> L)
- 3.7
- dn/dT used
- 3.75e−05 /K
- Source of dn/dT
- e, Jundt at λ, T
- Ring Γ, ng (template)
- 0.80, 2.30
Thesis example (10 W, 150 µm, 0.005 cm⁻¹, 20 mm, 100 °C, 5 W/(m K)): 61 mm from its own formula with the Moretti dne/dT at 632 nm; the thesis states about 100 mm, and which dn/dT it used is not stated.
L2 Coefficients, lens, ring shift
| Quantity | Value | Conditions | Source |
|---|---|---|---|
| dne/dT | 3.34×10−5 /K | 1523 nm, 300 K | Moretti et al. 2005, via Zhu 2021S |
| dne/dT | 3.75 / 4.01 / 4.89 ×10−5 /K | CLN, 1550 / 1064 / 633 nm, 25 °C; Jundt 1997 Sellmeier, recomputed | derived |
| dno/dT | 0.41 / 0.54 / 0.94 ×10−5 /K | CLN, 1550 / 1064 / 633 nm, 25 °C; data-sheet Sellmeier, recomputed | Crystal Technology 1999derived from V |
| dno/dT, dne/dT at 632 nm | (−1.7 + 6.9×10−3 T)×10−5 /K; (−2.6 + 22.4×10−3 T)×10−5 /K; at 300 K: 0.37 and 4.12×10−5 | T in K, 300-515 K | Schwesyg 2011, Eqs. 2.26-2.27 (Moretti 2005)S |
| Thermal conductivity | 3.92 W/(m K) CLN; 5.97 W/(m K) near-SLN | room temperature | Volk & Wöhlecke 2009, Table 1.1P-comp |
| Not for dn/dT | Gayer 2008 MgO:LN coefficients give anomalous dn/dT (e.g. −7.1×10−5 /K for MgO1-SLN ne at 1550 nm) | derived; excluded |
- Thermal lens (Schwesyg Eq. 2.28 S): f ≈ πw2Kth/(αPL dn/dT), valid for f ≫ L.
- Ring thermal shift: dλres/dT = λΓ(dneff/dT)/ng, with Γ and ng from the mode (templates in the figure).
- x-cut anisotropy: in x-cut TFLN the thermo-optic response depends on propagation angle and polarization through the mode's overlap with the o and e axes; a generalized analytical model exists (Shim et al. 2026reported).
- Athermal ring: a thin TiO2 cladding on an x-cut LN ring cancels the first-order thermo-optic coefficient at 20 °C; residual second order 0.37 pm/K2; resonance within 0.33 nm over −10 to 50 °C (Ling et al. 2020reported).
- High power: absorption heating and beam-quality loss reported in MgO:PPLN above 10 W pump; an absorption of 10−4 cm−1 already matters for cw singly resonant OPOs pumped at 10-20 W (Schwesyg p. 21 S).
Conflict. The thesis thermal-lens example (10 W, w = 150 µm, α = 0.005 cm−1, L = 20 mm, 100 °C, Kth = 5 W/(m K)) gives f = 61 mm with dne/dT at 632 nm and 373 K from the Moretti fit derived; the thesis states about 100 mm. Same order; which dn/dT the thesis used is not stated.
L3 Bistability and sources
- Thermal bistability (Carmon et al. 2004 reported (title)). Standard model used by the figure: absorbed power heats the ring, n rises, the resonance red-shifts; a laser swept toward longer wavelength drags the resonance along its flank until it drops off (triangular dip); swept toward shorter wavelength it jumps across the resonance (narrowed dip). Photorefraction in LN adds a slower term of opposite sign (Lin et al. 2021reported), with reported oscillation dynamics (Sun et al. 2017reported (title)) and self-starting soliton combs (He et al. 2019reported).
- dn/dT sources: Moretti 2005 (320-515 K, 632 and 1523 nm, interferometric; abstract read, table not read); Jundt 1997 (temperature-dependent ne Sellmeier; coefficients via a secondary). dno/dT disagrees by up to 2.5× between the data-sheet Sellmeier and the Moretti fit.
- Measurement: interferometric phase versus temperature on a plate; ring resonance tracking versus stage temperature, separated from optical self-heating by low probe power.
Ring sweep with photorefraction off; switch it on to compare with 4.3. The template model shows the shortened triangle; it does not produce the oscillations reported by Sun et al.
- sweep
- 1.00e+00 nm/s
- P
- 1.00e+00 mW
- thermal shift, max
- 1.01e+01 pm
- PR shift, max
- 0.00e+00 pm
- Tmin up / down
- 0.000 / 0.376
- QL, linewidth
- 5.00e+05, 3.10 pm
The thermal triangle
TFLN ring, radius 100 µm, 1550 nm laser swept across one resonance- Transmission
- 0.967
- Thermal shift, max
- +10.1 pm
- Photorefractive shift, max
- 0.0 pm
- Loaded Q, linewidth
- 5.00e+05, 3.10 pm
Sources
- Moretti et al. 2005L. Moretti, M. Iodice, F. G. Della Corte, I. Rendina, Temperature dependence of the thermo-optic coefficient of lithium niobate, from 300 to 515 K in the visible and infrared regions. Journal of Applied Physics 98 036101 (2005), doi:10.1063/1.1988987.Read: abstract (numbers via Zhu et al. 2021 and Schwesyg 2011, S)
- Jundt 1997D. H. Jundt, Temperature-dependent Sellmeier equation for the index of refraction, n_e, in congruent lithium niobate. Optics Letters 22 1553 (1997), doi:10.1364/OL.22.001553.Read: not read; coefficients via a secondary source (S)
- Crystal Technology 1999Crystal Technology Inc., LiNbO3 material properties, data sheet DC-12 8/99. (1999).Read: data sheet values via a secondary compilation
- Zhu et al. 2021Di Zhu, Linbo Shao, Mengjie Yu et al., Integrated photonics on thin-film lithium niobate. Advances in Optics and Photonics 13 242 (2021), doi:10.1364/AOP.411024.Read: secondary use only
- Carmon et al. 2004T. Carmon, L. Yang, K. J. Vahala, Dynamical thermal behavior and thermal self-stability of microcavities. Optics Express 12 4742 (2004), doi:10.1364/OPEX.12.004742.Read: title
- Lin et al. 2021Z. Lin, Z. Kang, P. Xu, Y. Tian, S. He, Turnkey generation of Kerr soliton microcombs on thin-film lithium niobate on insulator microresonators powered by the photorefractive effect. Optics Express 29 42932 (2021), doi:10.1364/OE.446527.Read: abstract
- Sun et al. 2017X. Sun, H. Liang, R. Luo, W. C. Jiang, X.-C. Zhang, Q. Lin, Nonlinear optical oscillation dynamics in high-Q lithium niobate microresonators. Optics Express 25 13504 (2017), doi:10.1364/OE.25.013504.Read: title
- He et al. 2019Yang He, Qi-Fan Yang, Jingwei Ling et al., Self-starting bi-chromatic LiNbO3 soliton microcomb. Optica 6 1138 (2019), doi:10.1364/OPTICA.6.001138.Read: arXiv abstract
- Ling et al. 2020J. Ling, Y. He, R. Luo, M. Li, H. Liang, Q. Lin, Athermal lithium niobate microresonator. Optics Express 28 21682 (2020), doi:10.1364/OE.398363.Read: abstract
- Shim et al. 2026Joonsup Shim, Seonghun Kim, Shengyuan Lu et al., Generalized Model of Anisotropic Thermo-Optic Response on Thin-Film Lithium Niobate Platform. ACS Photonics 13 2586-2596 (2026), doi:10.1021/acsphotonics.6c00117.Read: arXiv abstract
- Volk & Wöhlecke 2009Tatyana Volk, Manfred Wöhlecke, Lithium Niobate: Defects, Photorefraction and Ferroelectric Switching. Springer Series in Materials Science 115 (2009), doi:10.1007/978-3-540-70766-0.Read: selected chapters: Ch. 2.2 (pp. 14-19), Ch. 3 (pp. 51-61), Ch. 4 (pp. 75-77, 82-85, 94-97), Sec. 7.1.3 (p. 168)
- Schwesyg 2011Judith R. M.-L. Schwesyg, Interaction of light with impurities in lithium niobate crystals. Dr. rer. nat. dissertation, Universität Bonn (2011).Read: selected: Sec. 2.2.2-2.3.2 (pp. 10-21), Ch. 5 Sec. 5.1 (pp. 69-72), Sec. 5.4-5.5 (pp. 99-101)