3.6 Acousto-optics
L1 Phenomenon
A sound wave in a crystal is a moving grating of compressed and stretched regions, and the refractive index follows the strain (photoelastic effect). Light crossing it is diffracted and shifted in frequency by exactly the sound frequency. In LN the same crystal can launch the sound piezoelectrically, so a modulator, frequency shifter or deflector needs no glued-on transducer (acousto-optic effect).
Sweep the RF frequency: the diffracted beam swings like a scanner, the basis of an acousto-optic deflector, and the light frequency of the +1 order rises by exactly the RF frequency.
wavevectors to scale: kin + K = kout, |k| = 2πn/λ₀, K = 2π/Λ
K/k = 1.11e−1
- n (e), Zelmon 1997
- 2.1376
- v sound
- 6544.6 m/s
- Λ = v/f
- 6.54 µm
- θB inside
- 3.176°
- θB in air
- 6.801°
- deflection 2θB, air
- 13.602°
- shift of the +1 order
- +1.000 GHz
Crystal block, 200 µm wide
Bragg angle in air
- acoustic wavelength Λ
- 6.54 µm
- light frequency shift
- +1.000 GHz
- inside the crystal
- 3.176°
L2 Photoelastic tensor, figures of merit, devices
Photoelastic (strain-optic) relation (Weis & Gaylord 1985 Eq. 18 P). Nelson and Lax showed the independent variable is the displacement gradient, not only strain: rotations of volume elements contribute in birefringent crystals, so pijkl is not symmetric in kl for shear waves; in LN p44 = p55 has symmetric and antisymmetric parts, not resolved by the available data (Weis & Gaylord 1985 p. 200 P-comp).
3m form, eight independent coefficients p11, p12, p13, p14, p31, p33, p41, p44, with p22 = p11, p23 = p13, p24 = −p14, p32 = p31, p42 = −p41, p55 = p44, p56 = p41, p65 = p14, p66 = (p11 − p12)/2 (Weis & Gaylord 1985 Eq. 19 P). pIJ is not a symmetric matrix (p14 ≠ p41).
| Set | p11 | p12 | p13 | p14 | p31 | p33 | p41 | p44 | Status |
|---|---|---|---|---|---|---|---|---|---|
| Andrushchak 2009 | −0.021 | +0.060 | +0.172 | −0.052 | +0.141 | +0.118 | −0.109 | +0.121 | S |
| Avakyants 1976 (Set B) | −0.026 | +0.090 | +0.133 | −0.075 | +0.179 | +0.071 | −0.151 | +0.146 | P-comp |
| Krupych 2014 | −0.023 | +0.076 | +0.147 | +0.057 | +0.157 | +0.141 | +0.051 | +0.126 | S |
| Coquin (Pinnow 1971) | −0.020 | +0.080 | +0.130 | −0.080 | +0.170 | +0.070 | −0.150 | +0.120 | P-comp |
| TFLN fit, LN on sapphire (three components) | – | – | – | – | – | +0.038 | −0.038 | +0.085 | S |
Avakyants and Andrushchak at 633 nm; the wavelengths of the Coquin and Krupych sets are not recorded in the sources held. No set at 1550 nm is known; TFLN devices at 1550 nm reuse 633 nm values. Uncertainties of Andrushchak 2009: ±0.007 to ±0.029 (via Sarabalis et al. 2020 Table I).
Indirect (piezo-electro-optic) contribution. Strain makes a field through e, the field changes the index through r. It depends on the acoustic propagation direction and matters for p13 and p33: p13(primary) = p13(measured) − 0.043, p33(primary) = p33(measured) − 0.154 (Weis & Gaylord 1985 p. 201 P-comp; propagation direction not stated). Applied to Set B this gives p33(primary) of about −0.08 derived, so which p33 a model uses matters. The offsets are shown, not applied.
Figures of merit
LN, longitudinal wave along X with extraordinary light at 35° to y: n = 2.20, ρ = 4.7×10³ kg/m³, v = 6.57×10³ m/s (Dixon 1967 and Chang 1976 via Weis & Gaylord 1985 p. 201 P-comp).
| Quantity | Printed | From Eq. 2 with p implied by M2 | Status |
|---|---|---|---|
| M1 (m² s/kg) | 6.65×10−7 (Dixon 1967) | 6.64×10⁻⁷ | P-comp |
| M2 (s³/kg) | 6.99×10−15 (Dixon 1967) | input; p = 0.287 | P-comp |
| M4 (m4/(s kg)) | 62.9 (Chang 1976) | 63.0 | P-comp |
| M3 | printed “1.01×10−16 m s² kg” | 1.01×10⁻¹⁰ m s²/kg | U |
The four definitions with the stated n, ρ, v reproduce M1 and M4; the printed M3 exponent and unit are inconsistent with them, so the printed M3 is not used derived.
Bragg example. λ0 = 1550 nm, f = 1 GHz, X-longitudinal v = 6544.6 m/s: Λ = 6.54 µm and θB = 6.8° in air derived.
Integrated acousto-optics on LN. Collinear TE0-TE1 conversion by an SH0 wave at 440 MHz in a 1.25 µm wide suspended X-cut waveguide, up to 18% conversion (Sarabalis et al. 2021 reported); acousto-optic modulators in X-cut LN on sapphire (Sarabalis et al. 2020 reported); AO modulator VπL of 0.03 V cm in TFLN with chalcogenide, unsuspended (Wan et al. 2022 reported); a bulk-wafer longitudinal piezoelectric resonant photoelastic modulator (Atalar et al. 2022 S).
L3 Sign and frame pitfalls
1. Pair signs only within one frame. The p14 and p41 signs flip with c14 (and e22, d22) under a 180° rotation about Z. Never combine p14, p41 from one paper with c14, e22 from another without checking the frame.
2. What is known. Weis & Gaylord 1985 list Avakyants' p14, p41 < 0 next to Smith and Welsh's c14 > 0 in a paper that states the IRE frame, without saying it checked Avakyants' own frame; Krupych 2014 pairs c14 > 0 with p14, p41 > 0 (via Mys et al. 2015 S); Mytsyk et al. 2021 use S14 > 0 (c14 < 0) S, a frame that is non-standard for LN if d22 > 0 is imposed (inference). The common TFLN pairing (Kushibiki et al. c14 > 0 with Set B) matches the Weis & Gaylord compilation but is not confirmed at the primary level.
3. What a mismatch does. For a film with in-plane unit vector b (light polarization and dominant strain both along b), the longitudinal coefficient is p′bbbb = pijklbibjbkbl. On an X-cut film with b = (0, cos φ, sin φ), φ from +Y toward +Z derived:
| Set, X-cut | p′ at φ = 0, 45, 90, 135° | Maximum |
|---|---|---|
| Andrushchak 2009, A: as listed | −0.021, +0.304, +0.118, +0.143 | +0.304 at 44.3° |
| Andrushchak 2009, B: p14, p41 negated | −0.021, +0.143, +0.118, +0.304 | +0.304 at 135.7° |
| Avakyants 1976 (Set B), A: as listed | −0.026, +0.348, +0.071, +0.122 | +0.352 at 41.7° |
| Avakyants 1976 (Set B), B: p14, p41 negated | −0.026, +0.122, +0.071, +0.348 | +0.352 at 138.3° |
On X-cut the flip mirrors the optimum orientation from about 45° to about 135°; the magnitude is unchanged. On Y-cut (b = (cos φ, 0, sin φ)) the flip changes nothing (Andrushchak: maximum +0.230 at 50.7 and 129.3°; Set B maximum +0.238 at 48.3 and 131.7°). On Z-cut p′bbbb = p11 for every in-plane direction. Which orientation is right on X-cut depends on the unresolved pairing in item 2.
The Andrushchak values at 45 and 135°, 0.304 (X-cut) and 0.223 (Y-cut), equal the “p22′” values in the author's public 2018 note on photoelastic tensor rotation (outside5sigma.com, 2018 S), where the X-cut angle was relabelled from 45 to 135°. A p14/p41 sign or frame inconsistency produces such a relabelling; a change of the θ = 0 reference, also recorded in that note, is an alternative explanation (inference).
Toggle the film cut: on X-cut the two wafers disagree about the bright direction; on Y-cut they agree.
X-cut, φ from +Y toward +Z; radius |p′|
Y-cut, φ from +X toward +Z; radius |p′|
solid A: p₁₄, p₄₁ as listed (< 0); dashed B: negated
| X-cut φ | A | B |
|---|---|---|
| 0° | −0.021 | −0.021 |
| 45° | +0.304 | +0.143 |
| 90° | +0.118 | +0.118 |
| 135° | +0.143 | +0.304 |
- p′ at φ, A / B
- +0.3040 / +0.1430
- maximum, A
- +0.3041 at φ = 044.3°
- maximum, B
- +0.3041 at φ = 135.7°
Pairing A: p₁₄, p₄₁ as listed
Pairing B: p₁₄, p₄₁ negated
4. Optical wavelength. The Avakyants and Andrushchak sets are at 633 nm (Weis & Gaylord 1985 P-comp; Sarabalis et al. 2020 Table I S); no 1550 nm set is known.
5. Rotation (Nelson-Lax) term. For shear waves in a birefringent crystal it adds Δε terms proportional to (εii − εjj) times the rotation; an estimate for one LN nanobeam geometry put it below 4% of the photoelastic coupling (author's public 2018 note, outside5sigma.com S; unreviewed). Optomechanical coupling calculations on TFLN include moving-boundary and photoelastic terms; the rotation term is usually omitted.
References
| Source | Reference | Link |
|---|---|---|
| Weis & Gaylord 1985 | Weis & Gaylord, Applied Physics A Solids and Surfaces 37 191-203 (1985). Lithium niobate: Summary of physical properties and crystal structure | doi:10.1007/BF00614817 |
| Avakyants et al. 1976 | Avakyants, Kiselev & Shchitkov, Soviet Physics - Solid State 18 899 (1976) | none |
| Coquin 1971 | Coquin, cited in D. A. Pinnow, Handbook of Lasers (CRC) (1971) | none |
| Andrushchak et al. 2009 | Andrushchak et al., Journal of Applied Physics 106 073510 (2009). Complete sets of elastic constants and photoelastic coefficients of pure and MgO-doped lithium niobate crystals at room temperature | doi:10.1063/1.3238507 |
| Krupych et al. 2014 | Krupych, Savaryn & Vlokh, Applied Optics 53 B1 (2014). Precise determination of full matrix of piezo-optic coefficients with a four-point bending technique: the example of lithium niobate crystals | doi:10.1364/AO.53.0000B1 |
| Mys et al. 2015 | Mys, Applied Optics 54, 8176 (2015); arXiv:1508.01075 (2015) | none |
| Mytsyk et al. 2021 | Mytsyk et al., Crystals 11 1095 (2021). Photoelastic Properties of Trigonal Crystals | doi:10.3390/cryst11091095 |
| Sarabalis et al. 2020 | Sarabalis et al., APL Photonics 5 086104 (2020). Acousto-optic modulation in lithium niobate on sapphire | doi:10.1063/5.0012288 |
| Nelson & Lax 1970 | Nelson & Lax, Physical Review Letters 24 379-380 (1970). New Symmetry for Acousto-Optic Scattering | doi:10.1103/PhysRevLett.24.379 |
| Nelson & Lax 1971 | Nelson & Lax, Physical Review B 3 2778-2794 (1971). Theory of the Photoelastic Interaction | doi:10.1103/PhysRevB.3.2778 |
| Dixon 1967 | Dixon, Journal of Applied Physics 38 5149-5153 (1967). Photoelastic Properties of Selected Materials and Their Relevance for Applications to Acoustic Light Modulators and Scanners | doi:10.1063/1.1709293 |
| Chang 1976 | Chang, IEEE Transactions on Sonics and Ultrasonics 23 2-21 (1976). I. Acoustooptic Devices and Applications | doi:10.1109/T-SU.1976.30835 |
| Zelmon et al. 1997 | Zelmon, Small & Jundt, JOSA B 14 3319 (1997) | doi:10.1364/JOSAB.14.003319 |
| Sarabalis et al. 2021 | Sarabalis et al., Optica 8 477 (2021). Acousto-optic modulation of a wavelength-scale waveguide | doi:10.1364/OPTICA.413401 |
| Wan et al. 2022 | Wan et al., Light: Science & Applications 11 145 (2022). Highly efficient acousto-optic modulation using nonsuspended thin-film lithium niobate-chalcogenide hybrid waveguides | doi:10.1038/s41377-022-00840-6 |
| Atalar et al. 2022 | Atalar et al., Nature Communications 13 1526 (2022). Longitudinal piezoelectric resonant photoelastic modulator for efficient intensity modulation at megahertz frequencies | doi:10.1038/s41467-022-29204-9 |
| Jiang et al. 2019 | Jiang et al., Optica 6 845 (2019). Lithium niobate piezo-optomechanical crystals | doi:10.1364/OPTICA.6.000845 |
| Jiang 2018 | Jiang (2018). Rotation of photoelastic tensor and piezoelectric tensor (outside5sigma.com) | outside5sigma.com/tutorial/rotation-of-photoelastic-tensor-and-piezoelectric/ |